Photoactivation of triosmium dodecacarbonyl at 400 nm probed with time-resolved X-ray liquidography

  • Ki, Hosung
  • Kim, Tae Wu
  • Moon, Jiwon
  • Kim, Jungmin
  • Lee, Yunbeom
  • ... Kim, Jeongho
  • 외 8명
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초록

The photoactivation mechanism of Os-3(CO)(12) at 400 nm is examined with time-resolved X-ray liquidography. The data reveal two pathways: the vibrational relaxation following an internal conversion to the electronic ground state and the ligand dissociation to form Os-3(CO)(11) with a ligand vacancy at the axial position.

키워드

SOLUTION SCATTERING REVEALSM-3(CO)(12) MOS3(CO)12CLUSTERSDYNAMICSPHOTOCHEMISTRYPHOTOREACTIONSRU-3(CO)(12)REACTIVITYPHOTOLYSIS
제목
Photoactivation of triosmium dodecacarbonyl at 400 nm probed with time-resolved X-ray liquidography
저자
Ki, HosungKim, Tae WuMoon, JiwonKim, JungminLee, YunbeomHeo, JunKim, Kyung HwanKong, QingyuKhakhulin, DmitryNewby, GemmaKim, JoonghanKim, JeonghoWulff, MichaelIhee, Hyotcherl
DOI
10.1039/d2cc02438a
발행일
2022-06-30
유형
Article
저널명
Chemical Communications
58
53
페이지
7380 ~ 7383